低维功能材料与器件实验室
Lab for Low-Dimentional Functional Materials and Devices
徐宇曦 教授、博导
个人简介
徐宇曦，西湖大学工学院低维功能材料与器件实验室负责人，2007年6月本科毕业于武汉大学化学与分子科学学院，获理学学士学位；2011年6月博士毕业于清华大学化学系，获理学博士学位。随后在华盛顿大学、加州大学洛杉矶分校从事博士后研究，于2015年7月加入复旦大学高分子科学系/聚合物分子工程国家重点实验室任研究员/博导。于2019年4月底加入西湖大学工学院任研究员/博导（独立PI）。
学术成果
徐宇曦研究员课题组主要致力于新型高分子和石墨烯等低维功能材料的化学制备、可控组装复合及其在能源、催化、环境和生物医学中的应用。以第一/通讯作者在Nat. Commun.、Acc. Chem. Res.、J. Am. Chem. Soc.、Angew. Chem. Int. Ed.、Adv. Mater.等学术期刊上发表论文八十余篇，拓展了石墨烯功能化与组装、三维石墨烯宏观材料、二维合成高分子等研究方向，在国际上产生了较为广泛的影响，论文被Science、Nature等刊物他引两万多次（Google Scholar），其中单篇最高他引3500多次，曾入选过去十年中国被引用次数最高的十篇论文，14篇论文被ESI数据库收录为高被引论文，多篇论文被学术媒体和期刊作为封面文章和专题新闻亮点介绍，授权国内国际专利多项并转让一项给三星公司，获得2013年度教育部自然科学一等奖和2016年度国家自然科学二等奖（均为第二获奖人）、2019年中国化学会首届菁青化学新锐奖、2020年国家基金委优秀青年科学基金、2021 Young Innovator Award of Nano Research，入选上海市东方学者特聘教授（2015）、中国科协青年人才托举工程（2017）、浙江省万人计划青年拔尖人才（2020）、Clarivate Analytics全球高被引科学家（2018-2020）、Elsevier“中国高被引学者”（2019，2020）、英国皇家化学会会士（FRSC，2021），被学术期刊Adv. Mater. Interfaces和J. Mater. Chem. A分别遴选为2018 Hall of Fame和2018 Emerging Investigators，担任浙江省膜学会理事和国际期刊Nano Research的Young Star Editor。担任Nat. Chem.、JACS、Nat. Commun.、Angew. Chem.、Adv. Mater.等期刊审稿人。指导多名本科生和研究生获得国家奖学金和优秀毕业生称号，培养的毕业生去麻省理工学院等著名高校深造或者郑州大学等国内重点院校任教。
获得荣誉
-
获得2014年教育部自然科学一等奖(第二完成人)
-
获得2016年国家自然科学二等奖(第二完成人)
-
入选中国科协青年托举人才工程（2017）
-
入选Clarivate Analytics全球高被引科学家(2018-2020)
-
入选Elsevier中国高被引学者(2019)
-
获得2019年中国化学会首届菁青化学新锐奖
-
获得2020 Young Innovator Award of Nano Research
-
获得2020年国家自然科学基金优秀青年项目资助
-
上海市东方学者特聘教授、同济大学兼职教授、沙特国 王大学客座教授、浙江省膜学会理事
代表论文：
1. Jiwei Wang, Kaixi Wang, Yuxi Xu*, “Emerging Two-Dimensional Covalent and Coordination Polymers for Stable Lithium Metal Batteries: From Liquid to Solid”, ACS Nano 2021, DOI: 10.1021/acsnano.1c09194
2. Tian Sun, Yan Liang, Yuxi Xu*, “Rapid, Ordered Polymerization of Crystalline Semiconducting Covalent Triazine Frameworks”, Angew. Chem. Int. Ed. 2021, DOI: 10.1002/anie.202113926.
3. Kai Cui, Qingtao Wang, Zenan Bian, Gongming Wang, Yuxi Xu*, “Supramolecular Modulation of Molecular Conformation of Metal Porphyrins toward Remarkably Enhanced Multipurpose Electrocatalysis and Ultrahigh-Performance Zinc–Air Batteries”, Adv. Energy Mater. 2021, DOI: 10.1002/aenm.202102062
4. Congxu Wang, Hualei Zhang, Wenjia Luo, Tian Sun, Yuxi Xu*, “Ultrathin Crystalline Covalent-Triazine-Framework Nanosheets with Electron Donor Groups for Synergistically Enhanced Photocatalytic Water Splitting”, Angew. Chem. Int. Ed. 2021, 60, 25381-25390.
5. Xiaohua Qiao, Chaoqun Niu, Dankui Liao, Zhonghui Chen*, Lixia Sun*, Yuxi Xu*, “A Self-Growth Strategy for Simultaneous Modulation of Interlayer Distance and Lyophilicity of Graphene Layers toward Ultrahigh Potassium Storage Performance”, Adv. Funct. Mater. 2021, DOI: 10.1002/adfm.202105145.
6. Chaoqun Niu, Wenjia Luo, Chenmin Dai, Chengbing Yu, Yuxi Xu*, “High-Voltage-Tolerant Covalent Organic Framework Electrolyte with Holistically Oriented Channels for Solid-State Lithium Metal Batteries with Nickel-Rich Cathodes”, Angew. Chem. Int. Ed. 2021, 60, 24915-24923.
7. Kaixi Wang, Kwun Nam Hui, Kwan San Hui, Shaojun Peng*, Yuxi Xu*, “Recent Progress in Metal–Organic Framework/Graphene-Derived Materials for Energy Storage and Conversion: Design, Preparation, and Application”, Chem. Sci. 2021, 12, 5737-5766.
8. Peitao Xiao, Shuo Li, Chengbing Yu, Ying Wang*, Yuxi Xu*, “Interface Engineering between Metal-Organic Framework Nanocrystal and Graphene toward Ultrahigh Potassium-Ion Storage Performance”, ACS Nano, 2020, 14, 10210-10218.
9. Ke Li, Meiying Liang, Hao Wang, Xuehang Wang, Yanshan Huang, João Coelho, Sergio Pinilla, Yonglai Zhang, Fangwei Qi, Valeria Nicolosi*, Yuxi Xu*, “3D MXene Architectures for Efficient Energy Storage and Conversion”, Adv. Funct. Mater. 2020, 30, 2000842.
10. Zhonghui Chen, Xuhui An, Liming Dai*, Yuxi Xu*, “Holey Graphene-based Nanocomposites for Efficient Electrochemical Energy Storage”, Nano Energy 2020, 73, 104762.
11. Minmin Fan, Dankui Liao, Mohamed F. Aly Aboud, Imran Shakir, Yuxi Xu*, “A Universal Strategy toward Ultrasmall Hollow Nanostructures with Remarkable Electrochemical Performance”, Angew. Chem. Int. Ed. 2020, 59, 8247-8254.
12. Haiyan Duan, Pengbo Lyu, Jingjing Liu, Yanli Zhao, Yuxi Xu*, “Semiconducting Crystalline Two-Dimensional Polyimide Nanosheets with Superior Sodium Storage Properties”, ACS Nano, 2019, 13, 2473-2480.
13. Zhonghui Chen, Jiadong Chen, Fanxing Bu, Phillips O. Agboola, Imran Shakir*, Yuxi Xu*, “Double-Holey-Heterostructure Frameworks Enable Fast, Stable and Simultaneous Ultrahigh Gravimetric, Areal, and Volumetric Lithium Storage”, ACS Nano, 2018, 12, 12879-12887.
14. Fanxing Bu, Wenshu Chen, Jiajun Gu, Phillips O. Agboola, Najeeb Fuad Al-Khalli, Imran Shakir*, Yuxi Xu*, “Microwave-Assisted CVD-Like Synthesis of Dispersed Monolayer/Few-Layer N-Doped Graphene Encapsulated Metal Nanocrystals for Efficient Electrocatalytic Oxygen Evolution”, Chem. Sci. 2018, 9, 7009-7016.
15. Jingjing Liu, Yang Yang, Pengbo Lyu, Petr Nachtigall, Yuxi Xu*, “Few-Layer Silicene Nanosheets with Superior Lithium-Storage Properties”, Adv. Mater., 2018, 30, 1800838.
16. Peitao Xiao, Fanxing Bu, Ranran Zhao, Mohamed F. Aly Aboud, Imran Shakir*, Yuxi Xu*, “Sub-5 nm Ultrasmall Metal–Organic Framework Nanocrystals for Highly Efficient Electrochemical Energy Storage”, ACS Nano, 2018, 12, 3947-3953.
17. Jingjing Liu, Pengbo Lyu, Yu Zhang, Petr Nachtigall, Yuxi Xu*, “New Layered Triazine Framework/Exfoliated Two-Dimensional Polymer with Superior Sodium-Storage Properties”, Adv. Mater., 2018, 30, 1705401.
18. Runze Liu, Yu Zhang, Zhenjian Ning, Yuxi Xu*, “A Catalytic Microwave Process for Superfast Preparation of High-Quality Reduced Graphene Oxide”, Angew. Chem. Int. Ed. 2017, 56, 15677-15682.
19. Peitao Xiao, Fanxing Bu, Guanhui Yang, Yu Zhang, Yuxi Xu*, “Integration of Graphene, Nano Sulfur and Conducting Polymer into Compact Flexible Lithium-Sulfur Battery Cathode with Ultrahigh Volumetric Capacity and Superior Cycling Stability for Foldable Devices”, Adv. Mater., 2017, 29, 1703324.
20. Jingjing Liu, Wu Zan, Ke Li, Yang Yang, Fanxing Bu, Yuxi Xu*, “Solution Synthesis of Semiconducting Two-Dimensional Polymer via Trimerization of Carbonitrile”, J. Am. Chem. Soc., 2017, 139, 11666-11669.
21. Tiancai Jiang, Fanxing Bu, Xiaoxiang Feng, Imran Shakir*, Guolin Hao*, Yuxi Xu*, “Porous Fe2O3 Nanoframeworks Encapsulated within Three-Dimensional Graphene as High-Performance Flexible Anode for Lithium-Ion Battery”, ACS Nano, 2017, 11, 5140-5147.
22. Meng Wang, Xidong Duan, Yuxi Xu*, Xiangfeng Duan*, “Functional Three-Dimensional Graphene/Polymer Composites”, ACS Nano 2016, 10, 7231-7247.
23. Yuxi Xu, Gaoquan Shi, Xiangfeng Duan, “Self-Assembled Three-Dimensional Graphene Macrostructures: Synthesis and Applications in Supercapacitors”, Acc. Chem. Res. 2015, 48, 1666-1675.
24. Yuxi Xu, Chih-Yen Chen, Zipeng Zhao, Zhaoyang Lin, Xu Xu, Chain Lee, Xiangfeng Duan, “Solution Processable Holey Graphene Oxide and Its Derived Macrostructures for High-Performance Supercapacitors”, Nano Lett. 2015, 15, 4605-4610.
25. Yuxi Xu, Zhaoyang Lin, Xing Zhong, Ben Papandrea, Yu Huang, Xiangfeng Duan, “Solvated Graphene Frameworks as High-Performance Anodes for Lithium-Ion Batteries”, Angew. Chem. Int. Ed. 2015, 54, 5345-5350.
26. Yuxi Xu, Zhaoyang Lin, Xing Zhong, Xiaoqing Huang, Nathan O. Weiss, Yu Huang, Xiangfeng Duan, “Holey Graphene Frameworks for Highly Efficient Capacitive Energy Storage”, Nat. Commun. 2014, 5, 4554.
27. Yuxi Xu, Zhaoyang Lin, Xiaoqing Huang, Yang Wang, Yu Huang, Xiangfeng Duan, “Functionalized Graphene Hydrogels Based High-Performance Supercapacitors”, Adv. Mater. 2013, 25, 5779-5784.
28. Yuxi Xu, Zhaoyang Lin, Xiaoqing Huang, Yuan Liu, Yu Huang, Xiangfeng Duan, “Flexible Solid-State Supercapacitors Based on Three-Dimensional Graphene Hydrogel Films”, ACS Nano 2013, 7, 4042-4049.
29. Yuxi Xu, Qiong Wu, Yiqing Sun, Hua Bai, Gaoquan Shi, “Three-Dimensional Self-Assembly of Graphene Oxide and DNA into Multifunctional Hydrogels”, ACS Nano 2010, 4, 7358-7362.
30. Yuxi Xu, Kaixuan Sheng, Chun Li, Gaoquan Shi, “Self-Assembled Graphene Hydrogel via a One-Step Hydrothermal Process”, ACS Nano 2010, 4, 4324-4330.
31. Yuxi Xu, Lu Zhao, Hua Bai, Wenjing Hong, Chun Li, Gaoquan Shi, “Chemically Converted Graphene Induced Molecular Flattening of Porphyrin and Its Application for Optical Detection of Cadmium(II) Ions”, J. Am. Chem. Soc. 2009, 131, 13490-13497.
32. Yuxi Xu, Hua Bai, Gewu Lu, Chun Li, Gaoquan Shi, “Flexible Graphene Films via the Filtration of Water-Soluble Noncovalent Functionalized Graphene Sheets”, J. Am. Chem. Soc. 2008, 130, 5856-5857.